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From Gas Phase to Bulk — Photodissociation of Neutral Size Selected (HBr)n Clusters

Publication at Faculty of Mathematics and Physics |
2013

Abstract

We present results of photodissociation experiments with HBr molecules and clusters. The unique method of cluster size selection allow us to show main differences in hotodissociation dynamics between molecules, small clusters and large clusters prepared in expansions into vacuum.

The difference between the small cluster dynamics, which can be calculated by present ab initio methods and large cluster dynamics, which can be compared to bulk is crucial for understanding of the environmental effects on dissociation process.