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La-Substitution Effects on Multisite Ce Compound CePtGe2

Publication at Faculty of Mathematics and Physics |
2022

Abstract

The CePtGe2 compound, which shows antiferromagnetic transition at Neel temperature T-N = 3.8 K, has two crystallographically inequivalent Ce sites. Recently, the coexistence of a localized f-electron state at one of two Ce sites and an itinerant heavy f-electron state at the other Ce site has been suggested.

In this study, we have prepared polycrystalline samples of (Ce1-xLax)PtGe2 (x = 0 similar to 0.2) and have measured their electrical resistivity and magnetization. The specific heat for x = 0.2 has been measured also.

With increasing x, the downward bending of the temperature dependence of the resistivity and the cusp-type anomaly in the susceptibility associated with T-N shift to lower temperatures with a linear extrapolation of T-N directing to OK at x similar to 0.5. Also, the saturation magnetization decreases linearly with increasing x, pointing to the disappearance of magnetic moments at the same La concentration.

These results indicate that only the Ce ions with the localized f-electron are substituted by La ions. On the other hand, the transition from the anti ferromagnetic state to the ferromagnetic-like polarized magnetic state at a very weak magnetic field, which is comparable to that of conventional Ferrite magnets, was realized via the La-substitution.