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High harmonic generation in monolayer MoS2 controlled by resonant and near-resonant pulses on ultrashort time scales

Publikace na Matematicko-fyzikální fakulta |
2023

Tento text není v aktuálním jazyce dostupný. Zobrazuje se verze "en".Abstrakt

We report on experimental investigation of nonperturbative high harmonic generation (HHG) in monolayer MoS2 in the ultraviolet spectral region driven by mid-infrared light. We study how the HHG is influenced by pre-excitation of the monolayer using resonant and near-resonant pulses in a pump-probe-like scheme.

The resonant light creates high density exciton population. Due to ultrafast dephasing caused by electron-electron scattering, the HHG is suppressed in the presence of pre-excited carriers.

In the case of near-resonant excitation with photon energy below the exciton transition, the dynamics of the observed suppression of the HHG yield contains a fast component, which is a consequence of momentum scattering at carriers, which are excited by two-photon transition when the two pulses temporally overlap in the sample. This interpretation is supported by comparing the experimental data with theoretical calculations of the two-photon absorption spectrum of the MoS2 monolayer.

This work demonstrates a possibility to control HHG in low-dimensional materials on ultrashort timescales by combining the driving strong-field pulse with a weak near-resonant light.