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Terahertz Laser Pulse Boosts Interlayer Spin Transfer in Two-Dimensional van der Waals Magnetic Heterostructures

Publikace na Přírodovědecká fakulta |
2023

Tento text není v aktuálním jazyce dostupný. Zobrazuje se verze "en".Abstrakt

Light-induced ultrafast dynamics in two-dimensional (2D) magnetic systems demonstrate substantial advancements in spintronics. Here, using the real-time time-dependent density functional theory (rt-TDDFT), we applied laser pulses with various frequencies, from terahertz (THz) to optical pulse, to systematically study the interlayer spin transfer dynamics in 2D van der Waals nonmagnetic-ferromagnetic heterostructures, including graphene-Fe3GeTe2 (Gr/FGT) and silicene-Fe3GeTe2 (Si/FGT).

Our results demonstrate that low-frequency THz pulses are particularly effective in facilitating interlayer spin injection from the ferromagnetic FGT layers to the Si or Gr layers. On the contrary, high-frequency optical pulses exhibit a minimal influence on this process.

Such an effect is attributed to the low-frequency THz pulses inducing in-phase oscillations of the electron charge density around atomic centers, leading to a highly efficient interlayer spin transfer. Our results provide a new insight into ultrafast THz radiation control intralayer spin transfer and magnetic proximity dynamics in the 2D limit.

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